Even when running from the live CD / Pendrive, you must prefix your chmod command with sudo. So your steps will be like the following:
- boot from a live CD / Pendrive
- check whether your disk was already automounted (and where to). If not, mount it (see below)
- use
sudo chmod 0755 <path> to adjust the permissions
How to figure out where your disk is mounted: from a terminal window, run mount (without arguments). This will list up all mounted devices. Check for the type listed -- you can skip everything not using a "real file system" (your disk probably uses either ext3 or ext4 -- you can for sure skip things like proc, sysfs and the like). If something sounds promising (looking like /dev/sda1 on /media/sda1 type ext3), check its contents using ls /media/sda1 to see if it's that.
If it is not mounted, you can check with the /dev entries where the disk could be (using ls /dev/ |grep '/dev/sd to check for available devices; your disk should look like /dev/sdaX, /dev/sdbX or the like -- with X being a number). Compare this with the list of mounted devices. If it's not there, try to mount it and check its contents (as shown above). To mount it, first create a mountpoint, e.g. sudo mkdir /mnt/mydisk, then try to mount the device using mount /dev/sda1 /mnt/mydisk and check its contents using ls /mnt/mydisk.
Once you get the right disk there, you can go to change the permissions back on your usr dir: sudo chmod 0755 /mnt/mydisk/usr.
Now you still might be in trouble if you originally ran the chmod command recursively, using the -R parameter. In that case you can either try to fix each entry manually -- or you can go straight for a fresh install...
pkexecmethod in my answer (which you've marked as accepted) solve this problem for you? I've become convinced that, as Damien Roche and Oli have commented, this method does not actually work after asudo chmod -R 777 /usr/bincommand has successfully completed. Likesudo,pkexechas to be setuid root to work. (I'm not sure why, as it uses the polkit service, but it does.) However, I think I've heard other people say this has worked for them, which is curious! Had you pressed Ctrl+C before the777chmod command finished? – Eliah Kagan Aug 23 '14 at 1:10sudo chmod -R 777 /usr/bin, but only after logging into therootaccount. – iHowell Mar 14 '17 at 6:00